Full life cycle characterization strategies for spatiotemporal evolution of heterogeneous catalysts

作     者：Renyang Zheng Zaiku Xie 郑仁垟;谢在库

作者机构：China Petroleum&Chemical CorporationBeijing 100728China State Key Laboratory of Green Chemical Engineering and Industrial CatalysisSINOPEC Shanghai Research Institute of Petrochemical TechnologyShanghai 201208China 

基　　金：国家自然科学基金(22088101) 

出 版 物：《Chinese Journal of Catalysis》 (催化学报（英文）)

年 卷 期：2021年第42卷第12期

页      码：2141-2148页

摘      要：The sustainable development of the chemical industry requires novel and efficient catalysts and catalytic processes,especially eco-friendly and intrinsically safe *** idea is to improve the selectivity,activity,and stability of the catalyst in an appropriate ***,it is of great academic and industrial significance to conduct in-situ characterization of a working catalyst while testing its catalytic *** is beneficial for a comprehensive study on the dynamic evolution of the catalyst structure under real conditions,deepening the understanding of the structure-performance relationship of catalysts,and providing a scientific basis for the development of future generation catalytic *** far,it is still a great challenge to realize full life cycle characterization of heterogeneous catalysts from catalyst formation and function to deactivation under real world *** this mini review,we summarize the characterization strategies for heterogeneous catalysts,using zeolite,metal,and metal oxide catalysts as typical *** research strategies for the approximation of industrial conditions,multi-scale in-situ characterization devices,and computational modeling of realistic conditions should provide insight for the research and development of industrial catalysis.

主 题 词：Heterogeneous catalysis In-situ characterization Methanol-to-olefins Fischer-Tropsch synthesis Propane dehydrogenation 

学科分类：081705[081705] 08[工学] 0817[工学-轻工类] 080502[080502] 0805[工学-能源动力学] 

核心收录：

D　O　I：10.1016/S1872-2067(20)63786-X

馆 藏 号：203104903...