Fabrication of SnS_(2)/C_(3)N_(5), heterojunction photocatalyst for highly efficient hydrogen production and organic pollutant degradation
作者机构:Institute of Molecular ScienceKey Laboratory of Chemical Biology of Molecular Engineering of Education MinistryShanxi UniversityTaiyuan 030006China Scientific Instrument CenterShanxi UniversityTaiyuan 030006China
基 金:This project was supported by the Fundamental Research Program of Shanxi Province(202303021221058)
出 版 物:《燃料化学学报(中英文)》 (Journal of Fuel Chemistry and Technology)
年 卷 期:2025年第53卷第3期
页 码:336-347页
摘 要:The semiconductor photocatalysis are considered as one of the most promising candidates in hydrogen energy source and environmental remediation *** this paper,flower-shaped SnS,is successfully combined on g-C,Ns,and the well matching band structure successfully constitutes a new Type-II *** expected,the photocatalytic hydrogen production experiment showed that the quantity of hydrogen produced on 5% SnS_(2)/C_(3)N_(5)was 922.5μmol/(g.h),which is 3.6 times higher than that of pure g-C_(3)N_(5).Meanwhile,in photocatalytic degradation of methylene blue,5%SnS2/C,Ns composite material can degrade 95% of contaminants within 40 min,showing good photocatalytic degradation *** mechanism study indicates that SnS_(2)/C_(3)N_(5)heterojunction improves the photogenerated charge migration rate and reduces the electron-hole recombination rate,and effectively improves the photocatalytic performance of g-C_(3)N_(5).This work provides a new idea for designing C,Ns-based heterojunctions with efficient hydrogen production and degradation performance.
主 题 词:C_(3)N_(5) stannic disulfide photocatalysis hydrogen photodegradation
学科分类:081704[081704] 081705[081705] 07[理学] 070304[070304] 08[工学] 0817[工学-轻工类] 0703[理学-化学类]
核心收录:
D O I:10.1016/S1872-5813(24)60507-4
馆 藏 号:203157521...