摘要：A validated numerical model was established to simulate gas−liquid flow behaviors in the oxygen-enriched side-blown bath *** model included the slip velocity between phases and the gas thermal expansion *** modeling results were verified with theoretical correlations and experiments,and the nozzle-eroded states in practice were also involved in the *** comparison,it is confirmed that the thermal expansion effect influences the flow pattern significantly,which may lead to the backward motion of airflow and create a potential risk to production ***,the influences of air injection velocity and furnace width on airflow behavior were investigated to provide operating and design *** is found that the thin layer melt,which avoids high-rate oxygen airflow eroding nozzles,shrinks as the injection velocity increases,but safety can be guaranteed when the velocity ranges from 175 to 275 m/***,the isoline patterns and heights of thin layers change slightly when the furnace width increases from 2.2 to 2.8 m,indicating that the furnace width shows a limited influence on production safety.

摘要：Based on the building principle of additive manufacturing,printing orientation mainly determines the tribological properties of joint *** this study,we created a polyether-ether-ketone(PEEK)joint prosthesis using fused filament fabrication and investigated the effects of printing orientation on its tribological properties using a pin-on-plate tribometer in 25% newborn calf *** ultrahigh molecular weight polyethylene transfer film is formed on the surface of PEEK due to the mechanical capture of wear debris by the 3d-printed groove morphology,which is significantly impacted by the printing orientation of *** the printing orientation was parallel to the sliding direction of friction,the number and size of the transfer film increased due to higher steady *** transfer film protected the matrix and reduced the friction coefficient and wear rate of friction pairs by 39.13%and 74.33%,***,our findings provide a novel perspective regarding the role of printing orientation in designing knee prostheses,facilitating its practical applications.

摘要：The infamous type Ⅳ failure within the fine-grained heat-affected zone (FGHAZ) in G115 steel weldments seriously threatens the safe operation of ultra-supercritical (USC) power *** this work,the traditional thermo-mechanical treatment was modified via the replacement of hot-rolling with cold rolling,i.e.,normalizing,cold rolling,and tempering (NCT),which was developed to improve the creep strength of the FGHAZ in G115 steel *** NCT treatment effectively promoted the dissolution of preformed M_(23)C_(6)particles and relieved the boundary segregation of C and Cr during welding thermal cycling,which accelerated the dispersed reprecipitation of M_(23)C_(6) particles within the fresh reaustenitized grains during post-weld heat *** addition,the precipitation of Cu-rich phases and MX particles was promoted evidently due to the deformation-induced *** a result,the interacting actions between precipitates,dislocations,and boundaries during creep were reinforced *** this strategy,the creep rupture life of the FGHAZ in G115 steel weldments can be prolonged by 18.6%,which can further push the application of G115 steel in USC power plants.

摘要：The interface properties in two-dimensional(2d)layered materials and their van der Waals(vdW)homo-/heterostructures are of importance in both uncovering novel physical phenomena and optimizing device *** considerable research interest and enthusiasm direct toward the interlayer coupling in 2d homo-and heterostructures,there is limited research on the coupling at the 2d layered material-substrate *** limitation is due to the challenges in achieving direct ***,the coupling mechanisms at the 2d layered material-substrate interface is ambiguous,which needs greater *** this study,we have systematically investigated the interface coupling between monolayer WS_(2)and its supported substrates using high-temperature and high-vacuum in-situ raman spectroscopy through monitoring the low-frequency raman mode of monolayer WS_(2).Our findings reveal that both interfacial spacing and strain can significantly affect the coupling strength between the monolayer WS_(2)and the supported *** notably,we found that the strategic introduction of appropriate interfacial strain can effectively enhance the interface ***,we have succeeded in achieving effective regulation of the sample-substrate coupling via a convenient way of controlling the cooling process during *** findings contribute to a deeper understanding of the coupling correlation between 2d layered materials and substrates,which is of great significance for the design and optimization of high-performance devices based on 2d layered semiconductors.

摘要：Three-dimensional(3d)printing has attracted increasing research interest as an emerging manufacturing technology for devel-oping sophisticated and exquisite architecture through hierarchical *** has also been employed in various advanced industrial *** development of intelligent biomedical engineering has raised the requirements for 3d printing,such as flexible manufacturing processes and technologies,biocompatible constituents,and alternative ***,state-of-the-art 3d printing mainly involves inorganics or polymers and generally focuses on traditional industrial fields,thus severely limiting applications demanding biocompatibility and *** this regard,peptide architectonics,which are self-assembled by programmed amino acid sequences that can be flexibly functionalized,have shown promising potential as bioinspired inks for 3d ***,the combination of 3d printing and peptide self-assembly poten-tially opens up an alternative avenue of 3d bioprinting for diverse advanced ***,a small but innovative nation,has significantly contributed to 3d bioprinting in terms of scientific studies,marketization,and peptide architectonics,including modulations and applications,and ranks as a leading area in the 3d bioprinting *** review summarizes the recent progress in 3d bioprinting in Israel,focusing on scientific studies on printable components,soft devices,and tissue *** paper further delves into the manufacture of industrial products,such as artificial meats and bioinspired supramolecular architectures,and the mechanisms,physicochemical properties,and applications of peptide ***,Israel contributes significantly to the field of 3d bioprinting and should thus be appropriately recognized.

摘要：零差混频系统(Homodyne mixing system)对太赫兹超导动态电感探测器(Kinetic inductance detectors,KIds)性能表征具有重要的作用。然而,零差混频系统仍存在混频器不平衡性、测量系统集成、干扰信号等问题。作者设计新型的单通道零差混频硬件系统,结合软件算法实现了测量系统的集成化、IQ混频器不平衡性校准、KId的性能表征;同时实现了在VNA(vector network analyzer)CW模式下的KIds噪声测量;以及基于自相关算法的双通道零差混频硬件电路设计,有效地抑制了干扰信号。值得注意的是,这些研究成果被应用于表征KIds性能,对KIds阵列设计起到了重要的作用。

摘要：With the strict control of sulfur content in fuels,oxidative desulfurization(OdS),a promising desulphurization technology,needs to be continuously *** this study,we integrated multiple approaches(fabricating a porous structure,increasing phosphomolybdic acid(PMo)loading,improving amphiphilicity,and enhancing the intrinsic activity of PMo using a reductive framework)into PAF-54 carriers to improve OdS catalytic *** catalytic performance suggested that PAF-54 was not simply used as a carrier for PMo by physical *** the binding process,electron transfer between PAF-54 and PMo formed Mo^(5+)with superior catalytic *** to the presence of PAF-54,the catalytic activity of PMo as the active component qualitatively improved to achieve rapid and efficient *** importantly,we found that other nitrogen-rich porous organic polymers can also reduce some of Mo^(6+)in PMo during loading,and its formation mechanism was *** work provides a feasible strategy for designing highly efficient dOS catalysts.

摘要：为了探索Ar/N_(2)-Ar共溅射Ti掺杂对Ta_(2)O_(5)涂层光学性能和力学性能的影响,采用射频和直流磁控共溅射技术在玻璃基底表面制备了Ta_(2)O_(5)、N_(2)-Ta_(2)O_(5)、Ti-Ta_(2)O_(5)和N_(2)-Ti-Ta_(2)O_(5)涂层。利用X射线衍射仪(Xrd)、扫描电子显微镜(SEM)、原子力显微镜(AFM)表征了Ta_(2)O_(5)、N_(2)-Ta_(2)O_(5)、Ti-Ta_(2)O_(5)和N_(2)-Ti-Ta_(2)O_(5)涂层的微观结构和表面形貌;通过紫外可见分光光度计测试了涂层的光学参数;采用纳米压痕仪测试了涂层的硬度和杨氏模量。Xrd测试结果表明,Ta_(2)O_(5)、N_(2)-Ta_(2)O_(5)、Ti-Ta_(2)O_(5)和N_(2)-Ti-Ta_(2)O_(5)涂层主要以Ta_(2)O_(5)为主体的非晶相结构组成。SEM和AFM结果显示,沉积在玻璃基底上的涂层未出现大面积空隙,溅射粒子在基底表面均匀堆积生长,并且涂层沉积厚度基本一致,厚度误差在5%以内。分别引入N_(2)和Ti及N_(2)-Ti共掺杂,均可降低Ta_(2)O_(5)涂层的粗糙度。光学测试结果表明,分别引入N_(2)和Ti元素,可以提高Ta_(2)O_(5)涂层的平均透射率至81%以上,而N_(2)-Ti共掺杂制备的N_(2)-Ti-Ta_(2)O_(5)涂层平均透射率降低。力学测试结果显示,与Ta_(2)O_(5)涂层对比,N_(2)-Ta_(2)O_(5)和N_(2)-Ti-Ta_(2)O_(5)涂层的硬度显著增大,Ti-Ta_(2)O_(5)涂层硬度基本一致。弹性指数(H/E)和塑性指数(H^(3)/E^(2))表明,N_(2)-Ta_(2)O_(5)涂层和N_(2)-Ti-Ta_(2)O_(5)涂层具备更好的断裂韧性和抗塑性变形能力。在玻璃表面制备Ta_(2)O_(5)掺杂N_(2)和Ti元素的涂层,可以实现以N_(2)-Ta_(2)O_(5)涂层和N_(2)-Ti-Ta_(2)O_(5)涂层为代表的、同时具备优异光学性能和力学性能的多功能涂层。

摘要：在过去几十年中,将二氧化碳光还原转化为有用的化学燃料(甲烷、一氧化碳和甲醇等)受到了极大的关注.然而,由于光生电荷的复合速度快,二氧化碳和水分子的共吸附不足,目前的二氧化碳光还原系统的效率还远远不能令人满意.本文报道了在疏水碳纤维纸上构建一个紧密的二维/二维石墨相氮化碳@碘氧铋梯型(S型)异质结,用于高效的二氧化碳光还原.所制备的异质结具有良好的一氧化碳选择性(77.8%)和活性(458.0μmol h^(-1)m^(-2)).良好的光催化性能归因于良好设计的S型异质结结构,提高了电荷分离效率,以及形成了气-液-固三相界面,充分保证了二氧化碳和水的同时供给.这项工作为高效光催化二氧化碳还原系统的设计提供了新思路.

摘要：在流程工业关键变量预测领域,已有研究致力于将过程知识与大数据相结合,以实现更高的准确性,降低过拟合风险和提高可解释性.然而,现有工作存在准确的先验知识构建成本高、无法从丰富的数据中挖掘知识等问题,限制了这些方法在实际工业过程中的广泛应用.为了解决这些挑战,本文提出了一种基于知识协同进化的增强图卷积网络方法.首先,利用易获取的过程流图构建低成本的粗粒度流程知识.然后,在图卷积神经网络模型训练中引入图探索,实现知识更新.最后,为了降低知识复杂度并保持一致性,设计了一种知识过滤机制.所提出的方法在基准的脱丁烷塔工艺过程上进行了验证.实验结果表明,该方法具有出色的预测准确性,并获得高质量的新知识.