摘要：Trap-mediated energy loss in the buried interface with non-exposed feature constitutes one of the serious challenges for achieving high-performance perovskite solar cells(PSCs).Inspired by the adhesion mechanism of mussels,herein,three catechol derivatives with functional Lewis base groups,namely 3,4-Dihydroxyphenylalanine(DOPA),3,4-Dihydroxyphenethylamine(DA)and 3-(3,4-Dihydroxyphenyl)propionic acid(DPPA),were strategically *** molecules as interfacial linkers are incorporated into the buried interface between perovskite and SnO_(2) surface,achieving bilateral synergetic passivation *** crosslinking can produce secondary bonding with the undercoordinated Pb^(2+) and Sn^(4+) *** PSCs treated with DOPA exhibited the best performance and operational *** the DOPA passivation,a stabilized power conversion efficiency(PCE)of 21.5%was demonstrated for the planar *** 55 days of room-temperature storage,the unencapsulated devices with the DOPA crosslinker could still maintain 85%of their initial performance in air under relative humidity of-15%.This work opens up a new strategy for passivating the buried interfaces of perovskite photovoltaics and also provides important insights into designing defect passivation agents for other perovskite optoelectronic devices,such as light-emitting diodes,photodetectors,and lasers.

摘要：Mammals such as humans develop skeletal muscles composed of muscle fibers and connective tissue,which have mechanical properties that enable power output with three-dimensional motion when *** muscle-like actuators developed to date,such as the McKibben artificial muscle,often focus sole contractile elements and have rarely addressed the contribution of flexible connective tissue that forms an integral part of the structure and morphology of biological ***,we present a class of pneumatic muscle-like actuators,termed highly mimetic skeletal muscle(HimiSK)actuator,that consist of parallelly arranged contractile units in a flexible matrix inspired by ultrasonic measurements on skeletal *** contractile units act as a muscle fiber to produce active shortening force,and the flexible matrix functions as connective tissue to generate passive *** application of positive pressure to the contractile units can produce a linear contraction and *** this actuator,we assign different flexible materials as contractile units and a flexible matrix,thus forming five mold *** actuators feature three-dimensional motion on activation and present both intrinsic force-velocity and force-length characteristics that closely resebmle those of a biological *** output and tetanic force produced by harder contractile units improve the maximum output force by up to about 41.3%and the tetanic force by up to about 168%.Moreover,high displacement and velocity can be generated by a softer flexible matrix,with the improvement of maximum displacement up to about 33.3%and velocity up to about 73%.The results demonstrate that contractile units play a crucial role in force generation,while the flexible matrix has a significant impact on force transmission and deformation;the final force,velocity,displacement,and three-dimensional motion results from the interplay of contractile units,fluid and flexible *** approach introduces a m

摘要：The preparation of superhydrophobic or underwater superoleophobic interface materials has become a research hotspot because of their wide application in self-cleaning, drag reduction, oil-water separation, anti-oil pollution and so on. The unique wettability of organisms gives inspiration to design and create new interface materials. This review focuses on the recent research progress of femtosecond laser micro/nano fabrication for bioinspired superhydrophobic or underwater superoleophobic surfaces. This review starts with a presentation of the related background including the advantages of femtosecond laser and wettability theoretical basis. Then, organisms with unique wettability in nature, the preparation of superhydrophobic or underwater superoleophobic surfaces by femtosecond lasers on different materials, and their related important applications are introduced. Finally, the current challenges and future prospects with regard to this field are provided.

摘要：Dermal armor,such as fish scales or armadillo osteoderms,has been known to exhibit high performance and good flexibility defending against *** top layer of the dermal armor usually consists of a segmented hard bony *** soft inner layer composed of collagen fibers connects and holds the hard *** by the dermal armor of armadillos,bioinspired protection armor is studied for impact *** hexagonal scales tessellate the surface continuously and work as the hard bony layer protecting the soft inner layer from ***-high molecular weight polyethylene(UHMWPE)is used as the connectivity layer to support and hold the *** investigate the dynamic response of the bioinspired protection armor,drop weight impact tests are carried out.A finite element model is established to study the dynamic response of bioinspired protection *** impact process images captured by a high speed camera and the experimental data of drop hammer acceleration tests verify the validity of the numerical *** dynamic resistance behavior and the synergy effect of each part of the bioinspired protection armor combined with the protected objects are studied in detail by numerical *** results show that the bioinspired protection armor has marked energy absorption ability.A synergistic dissipation mechanism is activated in the impact process,which can dissipate impact energy and make the impact load distribution more *** UHMWPE between the outer layer and the soft substrate plays a significant role not only related to support and connection,but also for the force balance and energy *** mechanism of energy absorption of the bioinspired protection armor revealed in this paper can be taken as a new guideline for designing a novel protective armor.

摘要：As the main component of wearable electronic equipment,flexible pressure sensors have attracted wide attention due to their excellent sensitivity and their promise with respect to applications in health monitoring,electronic skin,and human-computer ***,it remains a significant challenge to achieve epidermal sensing over a wide sensing range,with short response/recovery time and featuring seamless conformability to the skin *** is critical since the capture of minute electrophysiological signals is important for health care *** this paper,we report the preparation of a nacre-like MXene/sodium carboxymethyl cellulose(CMC)nanocomposite film with a“brick-and-mortar”interior structure using a vacuum-induced self-assembly *** synergistic behavior of the MXene“brick”and flexible CMC“mortar”contributes to attenuating interlamellar self-stacking and creates numerous variable conductive pathways on the sensing *** resulted in a high sensitivity over a broad pressure range(i.e.,0.03-22.37 kPa:162.13 kPa^(-1);22.37-135.71 kPa:127.88 kPa^(-1);135.71-286.49 kPa:100.58 kPa^(-1)).This sensor also has a low detection limit(0.85 Pa),short response/recovery time(8.58 ms/34.34 ms),and good stability(2000 cycles).Furthermore,we deployed pressure sensors to distinguish among tiny particles,various physiological signals of the human body,space arrays,robot motion monitoring,and other related applications to demonstrate their feasibility for a variety of health and motion monitoring use cases.