摘要：Topological phase is an important development and unexplored degree of freedom of traditional band theory[1].Generally,it manifests in physics through the boundary states revealed by the bulkedge *** bulk topology implies various low-dimensional states at the boundary,giving extraordinary approaches to manipulate *** structure that encodes the band topology is the system associated with space–time evolution,such as Floquet topological insulator[2,3].Its quasistatic limit involves time-dependent dynamic adiabatic evolution[4,5].However,dynamic evolution is challenging as it requires fast modulation to overcome the dissipation of state before it is pumped from one edge to another[6].An alternative approach is to use an additional degree of freedom to replace the role of time,and an illuminating system is the weakly coupled waveguides,whose governing equation can be directly mapped to Schrodinger equation with time modulation replaced by wave propagation along the ***,such strategy has been largely explored to realize the pumping of topological boundary states in optics[7,8]and elastic wave[9,10].However,the strategy for acoustics is subtly different as the coupling of the acoustic waveguides is not weak for the fundamental waveguide *** exploring the possibility to realize two-dimensional(2D)topological acoustic pumping in a continuous regime remains an open question.

摘要：This vertically self‐pillared(VSP)structure extends the application range of traditional porous materials with facile mass/ion transport and enhanced reaction ***,we prepare a single crystal metal‐organic framework(MOF),employing the ZIF‐67 structure as a proof of concept,which is constructed by vertically self‐pillared nanosheets(VSP‐MOF).We further converted VSP‐MOF into VSP‐cobalt sulfide(VSP‐CoS2)through a sulfidation *** plays an important role in almost all battery technologies;for metallic batteries,lithium anodes exhibit a high theoretical specific capacity,low density,and low redox ***,during the half‐cell reaction(Li++e=Li),uncontrolled dendritic Li penetrates the separator and solid electrolyte interphase *** employed as a composite scaffold for lithium metal deposition,there are many advantage to using this framework:1)the VSP‐CoS2 substrate provides a high specific surface area to dissipate the ion flux and mass transfer and acts as a pre‐catalyst,2)the catalytic Co center favors the charge transfer process and preferentially binds the Li+with the enhanced electrical fields,and 3)the VSP structure guides the metallic propagation along the nanosheet 2D orientation without the protrusive *** these features enable the VSP structure in metallic batteries with encouraging performances.

摘要：To implement high quality tunneling injection quantum dot lasers, effects of primary factors on performance of the tunneling injection quantum dot lasers were investigated. The considered factors were tunneling probability, tun- neling time and carriers thermal escape time from the quantum well. The calculation results show that with increas- ing of the ground-state energy level in quantum well, the tunneling probability increases and the tunneling time decreases, while the thermal escape time decreases because the ground-state energy level is shallower. Longitudinal optical phonon-assisted tunneling can be an effective method to solve the problem that both the tunneling time and the thermal escape time decrease simultaneously with the ground-state energy level increasing in quantum well.

摘要：The design and synthesis of multifunctional nanocarriers for efficient synergistic cancer therapy have drawn great research interests in recent *** this work,a nanoplatform for chemo-photothermal therapy with targeting ligand was *** porous structured silica nanotubes(SNTs)with controllable lengths decorated with CuS nanoparticles(NPs)on the surface as photothermal agents were prepared and further conjugated with lactobionic acid groups as a cancer cell *** with average lengths of 40,55 and 150 nm were obtained and further functionalized as drug *** smallest bifunctional SNTs with targeting groups show good biocompatibility and highest cellular uptake for HepG2 *** release of doxorubicin hydrochloride(DOX)from the SNTs was dependent on the p H of the buffer solution and 808-nm near infrared(NIR)light *** integration of photothermal therapy(PTT)of CuS NPs and chemotherapy of anticancer drug leads to a better tumor inhibition effect than the individual therapy alone in vitro and in *** results demonstrate potential applications of the nanocomposites as vector for efficient chemo-photothermal therapy.

摘要：Daytime radiative cooling with high solar refection and mid-infrared emission offers a sustainable way for cooling without energy ***,so far sub-ambient daytime radiative coolers typically possess white/silver color with limited aesthetics and *** various colored radiative cooling designs have been pursued previously,multi-colored daytime radiative cooling to a temperature below ambient has not been realized as the solar thermal effect in the visible range lead to signifcant thermal ***,we demonstrate that photoluminescence(PL)based colored radiative coolers(PCRCs)with high internal quantum effciency enable sub-ambient full-color *** an example of experimental demonstration,we develop a scalable electrostatic-spinning/inkjet printing approach to realize the sub-ambient multi-colored radiative coolers based on quantum-dot *** unique features of obtained PCRCs are that the quantum dots atop convert the ultraviolet–visible sunlight into emitted light to minimize the solar-heat generation,and cellulose acetate based nanofbers as the underlayer that strongly refect sunlight and radiate thermal *** a result,the green,yellow and red colors of PCRCs achieve temperatures of 5.4–2.2℃ below ambient under sunlight(peak solar irradiance>740 Wm),*** the excellent cooling performance and scalable process,our designed PCRC opens a promising pathway towards colorful applications and scenarios of radiative cooling.

摘要：Coupled with anionic and cationic redox chemistry,Li-rich/excess cathode materials are prospective high-energy-density candidates for the next-generation Li-ion ***,irreversible lattice oxygen loss would exacerbate irreversible transition metal migration,resulting in a drastic voltage decay and capacity ***,a metastable layered Li-excess cathode material,T2-type Li_(0.72)[Li_(0.12)Ni_(0.36)Mn_(0.52)]O_(2),was developed,in which both oxygen stacking arrangement and Li coordination environment fundamentally differ from that in conventional O3-type layered *** means of the reversible Li migration processes and structural evolutions,not only can voltage decay be effectively restrained,but also excellent capacity retention can be achieved upon long-term ***,irreversible/reversible anionic/cationic redox activities have been well assigned and quantified by various in/ex-situ spectroscopic techniques,further clarifying the charge compensation mechanism associated with(de)*** findings of the novel T2 structure with the enhanced anionic redox stability will provide a new scope for the development of high-energy-density Li-rich cathode materials.

摘要：This paper discusses the analysis and design of a very thin slotless permanent magnet （PM） brushless motor whose stator laminations are manufactured from a single strip of steel that is edge wound into a spiral （like a ＂Slinky＂） and then fitted over the windings that are preformed on the outside surface of a non-conducting former. Analytical and finite element analysis （FEA） are used to determine the con- strained optimum dimensions of a motor used to drive a rim driven thruster in which the motor rotor is fit- ted onto the rim of the propeller and the stator is encapsulated in the thin Kort nozzle of the thruster. The paper describes the fabrication of a demonstrator motor and presents experimental results to validate the theoretical calculations. Experimental motor performance results are also reported and compared with those of a slotted motor that fits within the same active radial dimensions as the slotless motor. The slotless motor, which has longer active length and endwindings, and thicker magnets than the slotted motor, was found to be less efficient and more expensive （prototype cost） than the slotted machine.

摘要：Herein,we report the excellent De-NO_(x)performance of La0.7Sr0.3MnO3(LSM)perovskite-supported Pd catalysts(Pd-LSM)in alternating lean-burn/fuel-rich atmospheres using C3H6 as reductant and describe the in situ activation of the Pd catalysts via metal-support interaction(MSI)*** NO_(x)reduction conversion of the Pd-LSM catalyst increased significantly from 56.1%to 90.1%and the production of N2O was *** results demonstrated that this behavior was mainly attributed to the in situ transformation of Pd2+into Pd0 during the *** generated Pd0 species could readily activate the C3H6 reductant and achieve an eight-fold higher turnover frequency than Pd2+for the reduction of NO_(x).Moreover,excessive MSIs inhibited the in situ generation of Pd0,and thereby,lowered the De-NO_(x)activity of the catalyst even at high Pd *** addition,the Pd-LSM catalysts exhibited much higher S tolerance than conventional Al_(2)O_(3)-supported *** study provides a new approach for analyzing and designing highly active metal catalysts operated under dynamic alternating oxidizing/reducing atmospheric conditions.

摘要：Iron oxide supported Au nanomaterials are one of the most studied catalysts for low-temperature CO *** performance not only critically depends on the size of the supported Au nanoparticles(NPs)but also strongly on the chemical nature of the iron *** this study,Au NPs supported on iron oxide nanorods with different surface properties throughβ-FeOOH annealing,at varying temperatures,were synthesized,and applied in the CO *** characterizations of the interactions between Au NPs and iron oxides were obtained by X-ray diffraction,transmission electron microscopy(TEM),and X-ray photoelectron *** results indicate that the surface hydroxyl group on the Au/FeOOH catalyst,before calcination(Au/FeOOH-fresh),could facilitate the oxygen adsorption and dissociation on positively charged Au,thereby contributing to the low-temperature CO oxidation *** calcination at 200℃,under air exposure,the chemical state of the supported Au NP on varied iron oxides partly changed from metal cation to Au0,along with the disappearance of the surface OH ***/FeOOH with the highest Au0 content exhibits the highest activity in CO oxidation,among the as-synthesized ***,good durability in CO oxidation was achieved over the Au/FeOOH catalyst for 12 h without observable *** addition,the advanced identical-location TEM method was applied to the gas phase reaction to probe the structure evolution of the Au/iron oxide series of the catalysts and support structure.A Au NP size-dependent Ostwald ripening process mediated by the transport of Au(CO)x mobile species under certain reaction conditions is proposed,which offers a new insight into the validity of the structure-performance relationship.

摘要：Variable stiffness composite laminates(VSCLs)are promising in aerospace engineering due to their designable material properties through changing fiber angles and stacking *** to control the thermal postbuckling and nonlinear panel flutter motions of VSCLs,a full-order numerical model is developed based on the linear quadratic regulator(LQR)algorithm in control theory,the classical laminate plate theory(CLPT)considering von Kármán geometrical nonlinearity,and the first-order Piston *** critical buckling temperature and the critical aerodynamic pressure of VSCLs are parametrically *** location and shape of piezoelectric actuators for optimal control of the dynamic responses of VSCLs are determined through comparing the norms of feedback control gain(NFCG).Numerical simulations show that the temperature field has a great effect on aeroelastic tailoring of VSCLs;the curvilinear fiber path of VSCLs can significantly affect the optimal location and shape of piezoelectric actuator for flutter suppression;the unstable panel flutter and the thermal postbuckling deflection can be suppressed effectively through optimal design of piezoelectric patches.