摘要：Anthropogenic aerosols are effective radiative forcing agents that perturb the Earth’s climate. Major emission sources shifted from the western to eastern hemisphere around the 1980 s. An ensemble of single-forcing simulations with an Earth System Model reveals two stages of aerosol-induced climate change in response to the global aerosol increase for 1940–1980 and the zonal shift of aerosol forcing for 1980–2020, respectively. Here, using idealized experiments with hierarchical models, we show that the aerosol increase and shift modes of aerosol-forced climate change are dynamically distinct, governed by the inter-hemispheric energy transport and basin-wide ocean–atmosphere interactions, *** aerosol increase mode dominates in the motionless slab ocean model but is damped by ocean dynamics. Free of zonal-mean energy perturbation, characterized by an anomalous North Atlantic warming and North Pacific cooling, the zonal shift mode is amplified by interactive ocean dynamics through Bjerknes feedback. Both modes contribute to a La Ni?a-like pattern over the equatorial Pacific. We suggest that a global perspective that accommodates the evolving geographical distribution of aerosol emissions is vital for understanding the aerosol-forced historical climate change.

摘要：首先根据2000年环北京实际的精细下垫面布局资料(500m分辨率),按美国USGS陆面资料分类标准(25类)对其提供的全球30 s经纬分辨率(≈1 km)下垫面分类资料进行了更新设计.进而针对一个北京夏季暴雨过程,利用10:3.3km双向双重嵌套的MM5V3.6-Noah LSM陆气耦合模式进行24h数值对比试验,研究了北京精细下垫面信息引入对暴雨的影响.分析表明:新设计的陆面资料更真实地反映了环北京区域的下垫面结构,尤其针对北京城区面积迅增特征;同时还修正了原资料将亚洲中纬度区域落叶阔叶林下垫面类型归属为热带(或亚热带)稀疏大草原类型的问题.其在数值天气模式中的引入会对短期暴雨过程的发生发展产生重要影响.对此次暴雨主要降水中心的模拟,12h差值分布范围远达30km以上,中心值相对差异可达30%.研究发现在城市下垫面和大气相互间存在一个重要的相互影响机制,即由于城区面积的扩大会导致自然植被减少,进而会减少地表蒸发及相应局地大气水分供应、加深边界层高度并增强大气水汽混合,这不利于降水的发生发展.

摘要：利用MEGAN模式估算了珠三角地区2006年异戊二烯的排放情况,并设计了两组敏感性实验深入探讨了气象模拟误差对异戊二烯排放的影响.估算结果显示,2006年珠三角地区异戊二烯的排放量为95.56×106kg(以C计),且主要分布在珠三角地区周边植被覆盖较高的地方;受气象条件季节变化的影响,异戊二烯的排放表现出显著的季节和日变化特征,最大异戊二烯排放通量季节出现在夏季,为0.920t·km-2(以C计),最大排放速率均出现在13:00.敏感性实验结果显示,气象模拟误差能显著影响异戊二烯的排放,升高(降低)太阳辐射的输入,异戊二烯的排放量增加(减小)36.20%～50.70%(30.73%～41.88%),大于温度改变引起的排放量变化;升高(降低)气象输入并不会改变异戊二烯排放的日变化特征,但能显著影响排放速率的大小.上午8:00或下午17:00,异戊二烯排放速率的改变最为明显.