摘要：钙钛矿太阳能电池(PSCs)的界面接触缺陷是影响其性能的重要因素,会引发迟滞效应从而降低转换效率(PCE)并使器件运行稳定性恶化.界面材料通常被用于消除界面缺陷,然而设计兼具优越电荷传输和缺陷钝化能力的高效界面分子仍然面临挑战.本文研究了四种新型推-拉型富勒烯二聚体DC_(60)-R1-R2(R1=H或Cl,R2=H或MeO),并将其作为金属氧化物和钙钛矿之间的界面层.这些富勒烯二聚体之间的极性取代基决定了分子间的相互作用,DC_(60)-Cl-MeO由于其吸电子基团(-Cl)与给电子基团(-MeO)之间最强的电子推拉效应,表现出最佳的电荷传输和缺陷钝化能力.DC_(60)-Cl-MeO作为界面材料的未封装平面结构(FAPbI3)x(MAPbBr3)1-xPSC获得最高23.3%的PCE,且无迟滞现象,即使在高湿环境中储存500小时后仍能保持接近100%的初始效率.在一个太阳光强度下,无需任何封装或者惰性气体保护,钙钛矿太阳能电池在最大功率点连续运行的外推TS80寿命(效率下降到初始值的80%)从参比器件的0.5小时延长到1110小时.推-拉型富勒烯分子是极具潜力的钙钛矿太阳能电池界面材料.

摘要：The inter-agency government information sharing(IAGIS)plays an important role in improving service and efficiency of government ***,there is still no effective and secure way for data-driven IAGIS to fulfill dynamic demands of information sharing between government *** by blockchain and data mining,a data-driven framework is proposed for IAGIS in this ***,the blockchain is used as the core to design the whole framework for monitoring and preventing leakage and abuse of government information,in order to guarantee information ***,a four-layer architecture is designed for implementing the proposed ***,the classical data mining algorithms PageRank and Apriori are applied to dynamically design smart contracts for information sharing,for the purposed of flexibly adjusting the information sharing strategies according to the practical demands of government agencies for public management and public ***,a case study is presented to illustrate the operation of the proposed framework.

摘要：Aqueous Zn-iodine(Zn-I_(2))batteries have attracted extensive research interest as an emerging redox conversion energy storage system due to the low cost and high ***,the shuttling effects of polyiodides arising from incomplete redox conversion and inhomogeneous Zn plating on the Zn anode surface always hinder the commercial application of Zn-I_(2)*** this work,a two-birds-with-one-stone strategy is reported for long-life Zn-I_(2)*** on the strategy,the sulfonate-functionalized carbon fiber not only acts as the excellent iodine limiter to inhibit iodine species shuttling,but also as the uniform Zn plating guidance layer on the Zn anode surface to prevent the inhomogeneous deposition of Zn^(2+).Consequently,a superior cycling stability(a capacity of 124 mAh g^(-1)after 10,000 cycles at 5 A g^(-1))is *** calculations illustrate that sulfonate groups successfully induce charge redistribution on the carbon substrate,thereby strengthening the electronic interactions of the iodine species with the carbon *** charge-enriched sulfonate groups can guide the uniform deposition of Zn^(2+)through a strong Coulombic effect with Zn^(2+).This work gives a new perspective on the integrated design of cathodes and anodes for rechargeable batteries.

摘要：为了解决钎焊接头中脆性化合物的形成问题,我们设计了一种创新性的稀土改性还原氧化石墨烯增强AgCuTi复合钎料,进而获得了以Ag-Cu共晶为主要组织且脆性化合物生成量合适的钎焊接头。对比分析了有无稀土Ce改性的复合钎料的成分和显微组织,结果表明,经Ce改性后的还原氧化石墨烯在钎料中更加均匀分散。比较了分别采用有无Ce改性的钎料钎焊C/C复合材料-C/C复合材料接头的界面微观结构,并研究了石墨烯含量对接头组织和性能的影响。结果表明,由于经Ce改性的钎料中的还原氧化石墨烯分散性更好,从而细化了焊缝组织,且物相分布更均匀,使得接头的剪切强度明显提高。当石墨烯含量为0.5 wt.%时,使用Ce改性的钎料所得钎焊接头的平均剪切强度最高,为31.82 MPa,提高了50%。

摘要：This paper optimizes the buried channel charge-coupled device(BCCD) structure fabricated by complementary metal oxide semiconductor(CMOS) technology. The optimized BCCD has advantages of low noise, high integration and high image quality. The charge transfer process shows that interface traps, weak fringing fields and potential well between adjacent gates all cause the decrease of charge transfer efficiency(CTE). CTE and well capacity are simulated with different operating voltages and gap sizes. CTE can achieve 99.999% and the well capacity reaches up to 25 000 electrons for the gap size of 130 nm and the maximum operating voltage of 3 V.

摘要：The objective of steganography is to hide message securely in cover objects for secret *** to design a secure steganographic algorithm is still major challenge in this re-search *** this letter,developing secure steganography is formulated as solving a constrained IP(Integer Programming) problem,which takes the relative entropy of cover and stego distributions as the objective ***,a novel method is introduced based on BPSO(Binary Particle Swarm Optimization) for achieving the optimal solution of this programming *** results show that the proposed method can achieve excellent performance on preserving neighboring co-occurrence features for JPEG steganography.

摘要：Two non-ionic hydro-fluorocarbon hybrid surfactants with and without hydroxyl groups were synthesized and *** exhibited good thermal stability and superior surface *** was observed that the hydroxyl group had a profound effect on modifying the surface tension of their solutions and the morphology of the formed *** effect may be attributed to the rearranging of the alkane group from above the air/aqueous surface to below it and the disrupting of the interfacial water structure induced by the hydroxyl *** work provides a strategy to weaken the immiscibility between hydrocarbon and fluorocarbon chains by modifying their orientational structure at the interface,thus it is helpful for the design of surfactants with varied interfacial properties.

摘要：Because of their boundary-free and long-rangedisordered microstructure,Fe-based metallic glasses(MGs)exhibit an ultra-low pinning effect on the magnetic domain and unparalleled soft-magnetic properties[1-3],and thus are increasingly used in electric devices for the energy-saving and high-efficiency requirements[4,5].

摘要：The upcoming fifth-generation(5G)mobile communication with low-latency,high-speed and high-data-capacity[1]can realize innovative services such as remote intelligent medical care,smart cities,Internet of Vehicles,and ultra-high-definition video[2,3].Compared with current mobile communications,5G services require a 5G network with 1000 times the capacity and 10–100 times the data transmission rate[4].5G communication can also realize large-scale connections between people and machines[5].It will be the era of Internet of *** realization of the interconnection of all things is essentially the communication between the transmitting antenna and the receiving antenna.

摘要：A novel Cu?6.5Ni?1Al?1Si?0.15Mg?0.15Ce alloy with super-high strength was designed and its corrosion behavior in3.5%NaCl solution at25°C was investigated by the means of SEM observation,TEM observation and XPS *** alloy after solution treatment,80%cold rolling and aging at450°C for1h had the best comprehensive properties with hardness of HV314,electrical conductivity of19.4%IACS,tensile strength of1017MPa,and average annual corrosion rate of0.028mm/*** oxides and chloride products formed at first,followed by the formation of dyroxides *** alloy showed super-high strength,good electrical conductivity and corrosion resistant because Ni2Si hindered the precipitation of large NiAl at the grain boundary and the denickelefication of the alloy.