摘要：A VUV beamline at the Shanghai Synchrotron Radiation Facility （SSRF） for angle-resolved photoelectron spectroscopy （ARPES） measurements is designed. To increase the resolution and bulk sensitivity, a photon energy as low as 7 eV is desired. Because the reflectivity for p-polarized photons strongly decreases when the photon energy is below 30 eV, the design of a high flux beamline for low energy VUV photons is a challenge. This work shows a variable including angle Varied Line-space Plane-Grating Monochromator （VLPGM） with varied grating depth （VGD） which can achieve both high resolution and high flux with broad energy coverage.

摘要：All commercial electron spin polarimeters work in single channel mode, which is the bottleneck of researches by spin-resolved photoelectron spectroscopy. By adopting the time inversion antisymmetry of the magnetic field, we developed a multichannel spin polarimeter based on normal incident very low energy electron diffraction （VLEED）. The key point to achieve the multi-channel measurements is the spatial resolution of the electron optics. The test of the electron optics shows that the designed spatial resolution can be achieved and an image type spin polarimeter with 100 times 100, totally ten thousand channels is possible to be realized.

摘要：Existing technologies used to detect monosodium urate(MSU)crystals for gout diagnosis are not ideal due to their low sensitivity and complexity of *** purpose of this study was to explore whether aggregation-induced emission luminogens(AIEgens)can be used for highly specific imaging of MSU crystals to assist in the diagnosis of ***,we developed a series of luminogens(i.e.,tetraphenyl ethylene(TPE)-NH_(2),TPE-2NH_(2),TPE-4NH_(2),TPE-COOH,TPE-2COOH,TPE-4COOH,and TPE-Ketoalkyne),each of which was then evenly mixed with MSU ***,optimal fluorescence imaging of each of the luminogens was characterized by a confocal laser scanning microscope(CLSM).This approach was used for imaging standard samples of MSU,hydroxyapatite(HAP)crystals,and mixed samples with 1:1 mass ratio of MSU/*** also imaged samples from mouse models of acute gouty arthritis,HAP deposition disease,and comorbidities of ***,CLSM imaging results were compared with those of compensated polarized light microscopy,and we assessed the biosafety of TPE-Ketoalkyne in the RAW264.7 cell ***,CLSM time series and three-dimensional imaging were performed on MSU crystal samples from human gouty synovial fluid and *** a promising candidate for MSU crystal labeling,TPE-Ketoalkyne was found to detect MSU crystals accurately and rapidly in standard samples,animal samples,and human samples,and could precisely distinguish gout from HAP deposition *** work demonstrates that TPE-Ketoalkyne is suitable for highly specific and timely imaging of MSU crystals in gouty arthritis and may facilitate future research on MSU crystal-related diseases.

摘要：Fast charge transfer and anti-photocorrosion are two crucial factors for developing efficient, durable photoanodes for photoelectrochemical （PEC） cells. Reduced graphene oxide （RGO） is a promising photoanode element that can provide both of these. In this study, we elucidated the roles of RGO in the charge transfer and surface passivation of photoanodes by the precise design of a RGO-wrapped photoanode and examination of its PEC properties. Arrays of hetero-nanorods （HNRs） with three different designs were fabricated as photoanodes using RGO, CdSe nanoparticles （NPs）, and ZnO nanorods （NRs） as building blocks. CdSe@ZnO HNRs were prepared by decorating ZnO NRs with CdSe NPs. Finite-element analysis and experimental studies demonstrated that in the CdSe@ZnO HNRs, if only the ZnO NRs were wrapped by RGO, the conductivity between CdSe and ZnO was enhanced by RGO to shuttle charges. If RGO only surrounded the outside of the CdSe@ZnO HNRs, the corrosion was slowed owing to the passivation effect of RGO, which increased the electron lifetime of the photoanode. If both CdSe and ZnO were fully wrapped by RGO, the advantages of the two aforementioned cases were both obtained. RGO-wrapped CdSe@ZnO HNRs with position-controlled designs are promising photoanode materials with a high PEC efficiency, and the developed synthesis process can be applied to explore the design and fabrication of next-generation photoanodes using RGO as a buildin~ block.

摘要：In order to compare the sensitivity of short-range ensemble forecasts to different land-surface parameters in the South China region,three perturbation experiments related to the land surface model(LSM),initial soil moisture(ISM),and land–atmosphere coupling coefficient(LCC)were designed,and another control experiment driven by the Global Ensemble Forecast System(GEFS)was also *** ensemble members were initiated at 0000 UTC each day,and integrated for 24 h for a total of 40 days from the period 1 April to 10 May 2019 based on the Weather Research and Forecasting *** results showed that the perturbation experiment of the LSM(LSMPE)had the largest ensemble spread,as well as the lowest ensemble-mean root-mean-square error among the three sets of land-surface perturbed experiments,which indicated that it could represent more uncertainty and less *** ensemble spread of the perturbation experiment of the ISM(ISMPE)was generally less than that of LSMPE but greater than that of LCCPE(the perturbation experiment of the LCC).In particular,although the perturbation of the LCC could not produce greater spread,it had an effective influence on the intensity of ***,the ensemble spread of all the land-surface perturbed experiments was smaller than that of GEFSPE(the control experiment).Therefore,in future,land-surface perturbations and atmospheric perturbations should be combined in the design of ensemble forecasting systems to make the model represent more uncertainties.

摘要：Future climate change is usually projected by coupled earth system models under specific emission sce- narios designed by integrated assessment models （IAMs）, and this offline approach means there is no interaction between the coupled earth system models and the IAMs. This paper introduces a new method to design possible future emission scenarios and corresponding climate change, in which a simple economic and climate damage component is added to the coupled earth system model of Beijing Normal University （BNU-ESM）. With the growth of population and technological expertise and the declining emission-to-output ratio described in the Dynamic Inte- grated Climate-Economy model, the projected carbon emission is 13.7 Gt C, resulting in a 2.4℃ warming by the end of the twenty-first century （2080-2099） compared with 1980-1999. This paper also suggests the importance of the land and ocean carbon cycle in determining the CO2 con- centration in the atmosphere. It is hoped that in the near future the next generation of coupled earth system models that include both the natural system and the social dimension will be developed.

摘要：三维(3D)狄拉克半金属因其独特的拓扑能带结构及优异的光电性能在中/远红外波段的宽光谱光电探测领域具有巨大的应用潜力.然而,由于较大的暗电流,构建具有高信噪比(SNR)的3D狄拉克半金属宽光谱光电探测器仍面临很大挑战.本工作基于分子束外延生长的(Cd_(1-x)Zn_(x))_(3)As_(2)薄膜发展了一种超低器件噪声的3 D狄拉克半金属(Cd_(1-x)Zn_(x))_(3)As_(2)/Sb_(2)Se_(3)背靠背异质结光电探测器线阵.得益于有效的双异质结设计策略,该探测器可以实现从可见光(450 nm)到中红外(4.5μm)波段的室温高性能宽光谱探测器目标,其峰值SNR和D*分别可达104和5.2×10^(12)Jones,并具有相对较快的响应速度(~87.5μs).此外,不同探测器线列单元之间呈现出的稳定性、均匀性特征表明了其在未来应用于光迹实时跟踪等光电子器件中的可行性.该研究为基于3D狄拉克半金属材料制备具有超高SNR的高速宽光谱光电探测器提供了参考策略,展示了半金属在高速非制冷红外焦平面成像阵列探测器中的广阔前景.